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- W2892008423 endingPage "1160" @default.
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- W2892008423 abstract "The phase transition from swollen chains to polymer mesoglobules of an aqueous solution of poly(N-isopropylacrylamide) is investigated with kinetic small-angle neutron scattering with 50 ms time resolution in conjunction with millisecond pressure jumps across the coexistence line. The time-resolved study evidenced three distinct regimes: fractal clusters form during the first second and transform into compact mesoglobules. During the following ∼20 s, these grow by diffusion-limited coalescence. The final step consists of a slow growth characterized by an energy barrier of several kBT. The method opens opportunities for kinetic structural studies of multicomponent systems over wide length and time scales and gives a structural picture spanning from the chain collapse to mesoscopic phase separation." @default.
- W2892008423 created "2018-09-27" @default.
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- W2892008423 date "2018-09-11" @default.
- W2892008423 modified "2023-10-16" @default.
- W2892008423 title "Formation and Growth of Mesoglobules in Aqueous Poly(<i>N</i>-isopropylacrylamide) Solutions Revealed with Kinetic Small-Angle Neutron Scattering and Fast Pressure Jumps" @default.
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- W2892008423 doi "https://doi.org/10.1021/acsmacrolett.8b00605" @default.
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