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• W2892046382 endingPage "1803372" @default.
• W2892046382 startingPage "1803372" @default.
• W2892046382 abstract "Replacing noble-metal-based oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) electrocatalysts is the key to developing efficient Zn-air batteries (ZABs). Here, a homogeneous ternary Ni46 Co40 Fe14 nanoalloy with a size distribution of 30-60 nm dispersed in a carbon matrix (denoted as C@NCF-900) as a highly efficient bifunctional electrocatalyst produced via supercritical reaction and subsequent heat treatment at 900 °C is reported. Among all the transition-metal-based electrocatalysts, the C@NCF-900 exhibits the highest ORR performance in terms of half-wave potential (0.93 V) in 0.1 m KOH. Moreover, C@NCF-900 exhibits negligible activity decay after 10 000 voltage cycles with minor reduction (0.006 V). In ZABs, C@NCF-900 outperforms the mixture of Pt/C 20 wt% and IrO2 , cycled over 100 h under 58% depth of discharge condition. Furthermore, density functional theory (DFT) calculations and in situ X-ray absorption spectroscopy strongly support the active sites and site-selective reaction as a plausible ORR/OER mechanism of C@NCF-900." @default.
• W2892046382 created "2018-09-27" @default.
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• W2892046382 date "2018-09-14" @default.
• W2892046382 modified "2023-10-17" @default.
• W2892046382 title "A Ternary Ni₄₆ Co₄₀ Fe₁₄ Nanoalloy-Based Oxygen Electrocatalyst for Highly Efficient Rechargeable Zinc-Air Batteries" @default.
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• W2892046382 doi "https://doi.org/10.1002/adma.201803372" @default.
• W2892046382 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30216565" @default.
• W2892046382 hasPublicationYear "2018" @default.
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