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• W2892060029 abstract "A radical route to soot The chemical origin of soot is a persistent puzzle. It is clear that small hydrocarbon fragments formed in flames must aggregate into larger particles, but the initial driving force for aggregation remains a mystery. Johansson et al. combined theory and mass spectrometry to suggest a solution based on resonance-stabilized radicals (see the Perspective by Thomson and Mitra). Aromatics such as cyclopentadiene have a characteristically weak C–H bond because their cleavage produces radicals with extended spans of π-electron conjugation. Clusters thus build up through successive coupling reactions that extend conjugation in stabilized radicals of larger and larger size. Science , this issue p. 997 ; see also p. 978" @default.
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• W2892060029 date "2018-09-07" @default.
• W2892060029 modified "2023-10-11" @default.
• W2892060029 title "Resonance-stabilized hydrocarbon-radical chain reactions may explain soot inception and growth" @default.
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• W2892060029 doi "https://doi.org/10.1126/science.aat3417" @default.
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