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- W2892065842 abstract "The oxidation behavior of Ni/Al2O3 catalyst in CO2 plasma was investigated compared with CO2 thermal oxidation, aiming for providing new insight into oxidation-reduction cycle of plasma catalysis of dry methane reforming (DMR). Temperature programmed reaction spectrometry was applied to enable a quantitative analysis of gas consumption which is related to the oxidation and reduction of Ni/Al2O3 catalysts. The nonthermal plasma oxidation mechanism was further analyzed by Raman spectroscopy, showing the cross-sectional distribution of NiO over the 3 mm spherical catalyst pellets. Nonthermal plasma-excited CO2 oxidizes Ni only near the external surface of spherical pellets with 20 μm depth: both dielectric barrier discharge generation and plasma-excited species diffusion into the internal pores are inhibited. The partially oxidized Ni catalyst in the external surface would promote plasma-enabled oxidation-reduction cycle, which was further correlated with coke formation behavior in plasma catalysis of DMR." @default.
- W2892065842 created "2018-09-27" @default.
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- W2892065842 date "2018-10-01" @default.
- W2892065842 modified "2023-10-13" @default.
- W2892065842 title "Oxidation behavior of Ni/Al<sub>2</sub>O<sub>3</sub> catalyst in nonthermal plasma-enabled catalysis" @default.
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- W2892065842 doi "https://doi.org/10.1088/1361-6463/aae17d" @default.
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