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- W2892091475 abstract "The catalytic functionalization of unreactive CH bonds is an area of growing importance for the design of atomeconomical strategies to valuable organic molecules. However, due to the ubiquity of CH bonds in organic molecules,achieving perfect site-selectivity and high functional group tolerance has been one of the major challenges in this area. Inthis context, this dissertation outlines our efforts to develop key structure building CH functionalization reactions thatstreamline the construction of complex molecular skeletons based on the use of 2-pyridyl-containing directing groups.In particular, we have achieved:- The construction of CN bonds through a Cu-catalyzed cross-dehydrogenative coupling strategy.- The development of a Rh-catalyzed tandem process that involves the formation of CC and CX bonds.- A switchable site-selectivity through catalyst control in the direct Rh-catalyzed functionalization of molecules thatcontain distinct CH bonds.- A catalyst-controlled selectivity in the Rh-catalyzed C(sp2)–H functionalization with 1,3-diynes involving cyclizationcascade processes.- The Co-catalyzed alkyne annulation of N-containing arenes through CH/NH functionalization." @default.
- W2892091475 created "2018-09-27" @default.
- W2892091475 creator A5082419350 @default.
- W2892091475 date "2018-03-02" @default.
- W2892091475 modified "2023-09-24" @default.
- W2892091475 title "Novel c–h functionalization reactions assisted by 2-pyridyl-containing directing groups" @default.
- W2892091475 hasPublicationYear "2018" @default.
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