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- W2892155120 abstract "Measuring inelastic rates with partial wave resolution requires temperatures close to a Kelvin or below, even for the lightest molecule. In a recent experiment Perreault et al. [1] studied collisional relaxation of excited HD molecules in the v = 1, j = 2 state by para- and ortho-H2 at a temperature of about 1 K, extracting the angular distribution of scattered HD in the v = 1,j = 0 state. By state-preparation of the HD molecules, control of the angular distribution of scattered HD was demonstrated. Here, we report a first-principles simulation of that experiment which enables us to attribute the main features of the observed angular distribution to a single L = 2 partial-wave shape resonance. Our results demonstrate important stereodynamical insights that can be gained when numerically-exact quantum scattering calculations are combined with experimental results in the few-partial-wave regime." @default.
- W2892155120 created "2018-09-27" @default.
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- W2892155120 date "2018-09-11" @default.
- W2892155120 modified "2023-09-28" @default.
- W2892155120 title "Unraveling the Stereodynamics of Cold Controlled <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mi>HD</mml:mi><mml:mtext>−</mml:mtext><mml:msub><mml:mrow><mml:mi mathvariant=normal>H</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> Collisions" @default.
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- W2892155120 doi "https://doi.org/10.1103/physrevlett.121.113401" @default.
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