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- W2892230892 abstract "A series of unsupported MoS 2 , Co 9 S 8 , and Co-promoted MoS 2 catalysts have been synthesized by tuned impregnation and successive thermal annealing methods using a continuous flow of a mixture of H 2 and H 2 S gases. The resulting catalysts were evaluated in terms of their activity and selectivity for the hydrodesulfurization of dibenzothiophene (DBT) both in the absence and the presence of H 2 S. The inclusion of Co onto MoS 2 affected both the hydrogenation and direct desulfurization reactions, with the latter (production of biphenyl) being magnified to a much greater degree than the former. Interestingly, low cobalt/molybdenum ratio of ca. 0.05 of the catalyst exhibited outstanding promotion efficiency in the hydrodesulfurization reaction. However, as cobalt is added, the synergy effect drastically decreased. H 2 S in the reaction mixture led to a remarkable step up in the product from the direct desulfurization reaction route with the most notable increases occurring for the product from the hydrogenation reaction pathway. The HDS activity of such catalysts was much higher than that of the commercial CoMo/Al 2 O 3 . The promotion by H 2 S was discussed." @default.
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- W2892230892 date "2018-09-03" @default.
- W2892230892 modified "2023-10-14" @default.
- W2892230892 title "Highly Active Low Cobalt Content-Based Bulk MoS<sub>2</sub> Hydrodesulfurization Catalysts with a Unique Impact of H<sub>2</sub>S" @default.
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- W2892230892 doi "https://doi.org/10.1155/2018/8076534" @default.
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