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- W2892453199 abstract "Water electrolysis is among the simplest methods to generate hydrogen, which can be used as a clean and renewable energy source. Within this process, the oxidation of water into molecular oxygen is considered as the bottleneck reaction because it involves the transfer of four electrons toward the oxidation of a highly stable small molecule. Challenges in this area include the development of stable and effective electro- and photocatalysts that utilize readily available metal ions. Herein we report a copper–peptidomimetic complex as an electrocatalyst for water oxidation, which is both highly stable and efficient. Inspired by enzymatic catalysis, which is largely based on intramolecular cooperativity between a metal center and functional organic molecules located on one scaffold, we have designed and synthesized a peptoid trimer bearing a 2,2′-bipyridine (bipy) ligand, an −OH group, and a benzyl group. Both experimental and computational data reveal that binding of CuII to this peptoid in aqueous medium oc..." @default.
- W2892453199 created "2018-10-05" @default.
- W2892453199 creator A5001353917 @default.
- W2892453199 creator A5032058856 @default.
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- W2892453199 date "2018-09-28" @default.
- W2892453199 modified "2023-09-23" @default.
- W2892453199 title "A Copper-Peptoid as a Highly Stable, Efficient, and Reusable Homogeneous Water Oxidation Electrocatalyst" @default.
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- W2892453199 doi "https://doi.org/10.1021/acscatal.8b03661" @default.
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