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- W2892454844 abstract "Local structural heterogeneity is known to enhance the piezoelectric response of perovskite-based ferroelectrics. Here we investigate how this heterogeneity is affected by strong electric fields using dilute doped ${mathrm{Eu}}^{+3}$ ions as local structural probes. We make use of the extreme sensitivity of the $^{5}D_{0}ensuremath{rightarrow}^{7}F_{2}$ hypersensitive transition of ${mathrm{Eu}}^{+3}$ vis-`a-vis the asymmetric distribution of the ligand field around the doped ion to demonstrate that a strong electric field (poling) increases the overall low-symmetry regions on the local length scale in a ${mathrm{BaTiO}}_{3}$-based lead-free piezoceramic near the $P4mmtext{ensuremath{-}}Amm2$ polymorphic phase boundary (PPB). Our study suggests that the mandatory treatment of poling given to a ceramic to make it piezoactive also contributes to the microscopic mechanisms that improve the system's piezo-response." @default.
- W2892454844 created "2018-10-05" @default.
- W2892454844 creator A5015373130 @default.
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- W2892454844 date "2018-09-24" @default.
- W2892454844 modified "2023-09-23" @default.
- W2892454844 title "Synergistic role of poling in enhancing structural heterogeneity in perovskite piezoelectrics" @default.
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- W2892454844 doi "https://doi.org/10.1103/physrevb.98.094111" @default.
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