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• W2892625421 abstract "Tri-metallic nanowire catalysts combine the synergistic effect of multiple metals with the geometrical effect of nanowires, exhibiting better catalytic performance than composition-equivalent nanospherical catalysts. However, tri-metallic nanowires are not easily produced directly because of the participation of multiple precursors and the difficulty of selecting capping agents. Herein, we develop a one-pot, two-step synthetic strategy, producing tri-metallic Au/PdPt core/shell nanowires. Moreover, the PdPt shell is an alloy composed of nanoparticles, and its Pd : Pt atomic ratio is easily adjusted by controlling reaction time. The formation of Au/PdPt nanowires is attributed to the initial formation of Au/Pd core/shell nanowire and subsequent galvanic replacement between Pd shell and PtCl62−. As-prepared Au/PdPt nanowires show composition- and structure-dependent catalytic activity and durability for the electrooxidation of methanol and ethanol, and the Suzuki coupling reaction. Optimized Au/Pd63Pt37 nanowire, due to its proper Pd : Pt atomic ratio and porosity of the PdPt shell, exhibits excellent catalytic activity and durability towards methanol and ethanol electrooxidation, ∼18 and 11 times in the specific activity better than that of commercial state-of-the-art Pt/C catalyst, respectively. Moreover, Au/Pd63Pt37 nanowire shows the superior catalytic performance in Suzuki coupling reaction, ∼96 % at yield, far better than commercial state-of-the-art Pd/C catalyst." @default.
• W2892625421 created "2018-10-05" @default.
• W2892625421 creator A5039747472 @default.
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• W2892625421 date "2018-10-16" @default.
• W2892625421 modified "2023-10-16" @default.
• W2892625421 title "Self‐Supported Composition‐Tunable Au/PtPd Core/Shell Tri‐Metallic Nanowires for Boosting Alcohol Electrooxidation and Suzuki Coupling" @default.
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• W2892625421 doi "https://doi.org/10.1002/celc.201801255" @default.
• W2892625421 hasPublicationYear "2018" @default.
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