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• W2892662726 abstract "Mechanical bonds are known to efficiently absorb mechanical energy at low forces, but their behavior at high forces is unknown. Here we investigate the impact of a mechanical bond on the rate of activation of a Diels–Alder mechanophore. Using a combination of experimental and computational techniques, we found that the rate of a retro-Diels–Alder reaction under tension is decreased when the mechanophore is embedded in the axle of a rotaxane due to the presence of a competing high-stress region at the junction between the macrocycle and the axle." @default.
• W2892662726 created "2018-10-05" @default.
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• W2892662726 date "2018-09-24" @default.
• W2892662726 modified "2023-09-25" @default.
• W2892662726 title "Impact of a Mechanical Bond on the Activation of a Mechanophore" @default.
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• W2892662726 doi "https://doi.org/10.1021/jacs.8b08590" @default.
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• W2892662726 hasPublicationYear "2018" @default.
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