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- W2892677612 abstract "Abstract We recently developed a novel chiral catalyst‐directed dynamic kinetic diastereoselective acylation of hemiacetals for the synthesis of carbohydrates. In this update, we describe a catalytic method for the dynamic kinetic enantioselective acylation of 2‐chromanols using benzotetramisole derived catalysts. High yields and enantiomeric excesses were obtained for a broad range of acylated 2‐chromanols, which are important intermediates for the synthesis of various bioactive pharmaceuticals. We hypothesize that the high stereoselectivity of the reaction originates from a novel cation‐ n interaction between the chromanol substrate and the acylated catalyst. magnified image" @default.
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- W2892677612 date "2018-10-30" @default.
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- W2892677612 title "Organocatalyst-Mediated Dynamic Kinetic Enantioselective Acylation of 2-Chromanols" @default.
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- W2892677612 doi "https://doi.org/10.1002/adsc.201800994" @default.
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