FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2892709249> ?p ?o ?g. }

• W2892709249 endingPage "22896" @default.
• W2892709249 startingPage "22892" @default.
• W2892709249 abstract "To predict the radiative forcing of clouds it is necessary to know the rate with which ice homogeneously nucleates in supercooled water. Such rate is often measured in drops to avoid the presence of impurities. At large supercooling small (nanoscopic) drops must be used to prevent simultaneous nucleation events. The pressure inside such drops is larger than the atmospheric one by virtue of the Laplace equation. In this work, we take into account such pressure raise in order to predict the nucleation rate in droplets using the TIP4P/Ice water model. We start from a recent estimate of the maximum drop size that can be used at each supercooling avoiding simultaneous nucleation events [Espinosa et al. J. Chem. Phys., 2016]. We then evaluate the pressure inside the drops with the Laplace equation. Finally, we obtain the rate as a function of the supercooling by interpolating our previous results for 1 and 2000 bar [Espinosa et al. Phys. Rev. Lett. 2016] using the Classical Nucleation Theory expression for the rate. This requires, in turn, interpolating the ice-water interfacial free energy and chemical potential difference. The TIP4P/Ice rate curve thus obtained is in good agreement with most droplet-based experiments. In particular, we find a good agreement with measurements performed using nanoscopic drops, that are currently under debate. The successful comparison between model and experiments suggests that TIP4P/Ice is a reliable model to study the water-to-ice transition and that Classical Nucleation Theory is a good framework to understand it." @default.
• W2892709249 created "2018-10-05" @default.
• W2892709249 creator A5027678138 @default.
• W2892709249 creator A5031891035 @default.
• W2892709249 creator A5088034473 @default.
• W2892709249 date "2018-09-27" @default.
• W2892709249 modified "2023-10-13" @default.
• W2892709249 title "Homogeneous Ice Nucleation Rate in Water Droplets" @default.
• W2892709249 cites W1570025454 @default.
• W2892709249 cites W1571663278 @default.
• W2892709249 cites W1587101236 @default.
• W2892709249 cites W1633474379 @default.
• W2892709249 cites W1720499737 @default.
• W2892709249 cites W1969009815 @default.
• W2892709249 cites W1973590037 @default.
• W2892709249 cites W1981445094 @default.
• W2892709249 cites W1993436181 @default.
• W2892709249 cites W1994509642 @default.
• W2892709249 cites W1997615594 @default.
• W2892709249 cites W2014476086 @default.
• W2892709249 cites W2019396959 @default.
• W2892709249 cites W2022164742 @default.
• W2892709249 cites W2029243935 @default.
• W2892709249 cites W2047137396 @default.
• W2892709249 cites W2047190797 @default.
• W2892709249 cites W2048752444 @default.
• W2892709249 cites W2051827732 @default.
• W2892709249 cites W2054600704 @default.
• W2892709249 cites W2057846671 @default.
• W2892709249 cites W2074117796 @default.
• W2892709249 cites W2084177570 @default.
• W2892709249 cites W2090873013 @default.
• W2892709249 cites W2090928326 @default.
• W2892709249 cites W2100365896 @default.
• W2892709249 cites W2104248732 @default.
• W2892709249 cites W2127103267 @default.
• W2892709249 cites W2131980091 @default.
• W2892709249 cites W2278422378 @default.
• W2892709249 cites W2295294437 @default.
• W2892709249 cites W2328437366 @default.
• W2892709249 cites W2332699766 @default.
• W2892709249 cites W2336157959 @default.
• W2892709249 cites W2523571407 @default.
• W2892709249 cites W2525806282 @default.
• W2892709249 cites W2546291266 @default.
• W2892709249 cites W2556528070 @default.
• W2892709249 cites W2609724571 @default.
• W2892709249 cites W2767311213 @default.
• W2892709249 cites W2788083588 @default.
• W2892709249 cites W3100387547 @default.
• W2892709249 cites W3123608039 @default.
• W2892709249 cites W3168730743 @default.
• W2892709249 doi "https://doi.org/10.1021/acs.jpcc.8b04788" @default.
• W2892709249 hasPublicationYear "2018" @default.
• W2892709249 type Work @default.
• W2892709249 sameAs 2892709249 @default.
• W2892709249 citedByCount "24" @default.
• W2892709249 countsByYear W28927092492018 @default.
• W2892709249 countsByYear W28927092492019 @default.
• W2892709249 countsByYear W28927092492020 @default.
• W2892709249 countsByYear W28927092492021 @default.
• W2892709249 countsByYear W28927092492022 @default.
• W2892709249 countsByYear W28927092492023 @default.
• W2892709249 crossrefType "journal-article" @default.
• W2892709249 hasAuthorship W2892709249A5027678138 @default.
• W2892709249 hasAuthorship W2892709249A5031891035 @default.
• W2892709249 hasAuthorship W2892709249A5088034473 @default.
• W2892709249 hasBestOaLocation W28927092492 @default.
• W2892709249 hasConcept C112964491 @default.
• W2892709249 hasConcept C119049451 @default.
• W2892709249 hasConcept C121332964 @default.
• W2892709249 hasConcept C122409099 @default.
• W2892709249 hasConcept C147597530 @default.
• W2892709249 hasConcept C153294291 @default.
• W2892709249 hasConcept C185592680 @default.
• W2892709249 hasConcept C18762648 @default.
• W2892709249 hasConcept C188721877 @default.
• W2892709249 hasConcept C192562407 @default.
• W2892709249 hasConcept C2780393986 @default.
• W2892709249 hasConcept C57879066 @default.
• W2892709249 hasConcept C59593255 @default.
• W2892709249 hasConcept C61048295 @default.
• W2892709249 hasConcept C7772457 @default.
• W2892709249 hasConcept C8892853 @default.
• W2892709249 hasConcept C97355855 @default.
• W2892709249 hasConceptScore W2892709249C112964491 @default.
• W2892709249 hasConceptScore W2892709249C119049451 @default.
• W2892709249 hasConceptScore W2892709249C121332964 @default.
• W2892709249 hasConceptScore W2892709249C122409099 @default.
• W2892709249 hasConceptScore W2892709249C147597530 @default.
• W2892709249 hasConceptScore W2892709249C153294291 @default.
• W2892709249 hasConceptScore W2892709249C185592680 @default.
• W2892709249 hasConceptScore W2892709249C18762648 @default.
• W2892709249 hasConceptScore W2892709249C188721877 @default.
• W2892709249 hasConceptScore W2892709249C192562407 @default.
• W2892709249 hasConceptScore W2892709249C2780393986 @default.
• W2892709249 hasConceptScore W2892709249C57879066 @default.
• W2892709249 hasConceptScore W2892709249C59593255 @default.

• next