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- W2892872592 abstract "We present ultrafast optical pump-probe and ultrafast x-ray diffraction measurements of the charge density wave dynamics in ${mathrm{SmTe}}_{3}$ at 300 K. We performed ultrafast x-ray diffraction measurements at the Linac Coherent Light Source to directly probe the dynamics of the finite-wave-vector order parameter. The dynamics reveal coherent oscillations at $ensuremath{sim}1.6$ THz that become overdamped with increasing fluence. We identify this oscillation with the lattice component of the amplitude mode. Furthermore, our data allow for a clear identification of the amplitude mode frequency in the optical pump-probe data. In both measurements, the system reaches the symmetric phase at high fluence, where the order parameter vanishes and the response (reflectivity and x-ray intensity) is quadratic in the order parameter. This is observed in the x-ray diffraction as a small overdamped modulation near zero intensity. Similar overdamped features are observed in the optical reflectivity at high fluence. A time-dependent Ginzburg-Landau model captures qualitatively the essential features of the experimental observations." @default.
- W2892872592 created "2018-10-05" @default.
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- W2892872592 date "2019-03-28" @default.
- W2892872592 modified "2023-10-14" @default.
- W2892872592 title "Coherent order parameter dynamics in <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mi>SmTe</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:math>" @default.
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- W2892872592 doi "https://doi.org/10.1103/physrevb.99.104111" @default.
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