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• W2892901029 abstract "Many natural materials have helical or twisting shapes. Herein, we show the formation of helical fibers with the lengths of micrometers by the evaporation-driven self-assembly on silicon wafers of functionalized cellulose nanowhiskers (CNWs) with surface-attached acyl chains. The self-assembly process and the final helical structures were affected by parameters including the wettability of substrates, dispersing solvents, the amount of 10-undecenoyl groups, the crystallinity, the dimension of CNWs, and the length of acyl chains. In particular, surface-acylated CNWs with a certain amount of 10-undecenoyl groups (ca. 3.52 mmol g−1), an appropriate crystallinity (ca. 40 %), a length of about 135 nm, and a diameter of around 4 nm, preferentially self-assembled into explicit left-handed helical fibers from their THF suspensions on wafers. Thus, we showed novel particular self-assembly behaviors of surface-acylated CNWs, and we expanded the materials spectrum for the construction of helical structures." @default.
• W2892901029 created "2018-10-05" @default.
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• W2892901029 date "2018-11-11" @default.
• W2892901029 modified "2023-10-18" @default.
• W2892901029 title "Helical Fibers via Evaporation-Driven Self-Assembly of Surface-Acylated Cellulose Nanowhiskers" @default.
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• W2892901029 doi "https://doi.org/10.1002/anie.201808250" @default.
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