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• W2892924457 abstract "Abstract High-purity hydrogen to be fed directly to a PEMFC was produced by carrying out natural gas steam reforming under moderate operating conditions in a Pd-Au composite membrane reactor packed with a commercial Ni-based catalyst. The Pd-Au composite membrane with a thickness of approximately 12 µm was fabricated by using both electroless and electroplating techniques to deposit Pd and Au layers, respectively, over a porous stainless-steel support. After annealing, the membrane showed a hydrogen permeance of 1.30 × 10−3 mol/s-m2-Pa0.5 at 450 °C, and near-infinite ideal selectivity of H2/Ar at pressures lower than 300 kPa and at temperatures lower than 400 °C. The natural gas reforming reaction was performed at 450 °C with a steam-to-methane ratio of 3.5 and gas hourly space velocity of 2600 h−1 at different operating pressures varying from 100 kPa to 300 kPa. As a comparison, the steam methane reforming reaction was also carried out at the same operating conditions. The natural gas reforming reaction showed better performance than the steam methane reforming reaction and reached > 80% conversion of the higher hydrocarbons and almost 65% of hydrogen recovery at 450 °C and 300 kPa. High-purity hydrogen was obtained in all the experimental tests. No coke formation was observed. Post-reaction analysis of the membrane is discussed via scanning electron microscope and energy-dispersive X-ray spectroscopy." @default.
• W2892924457 created "2018-10-05" @default.
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• W2892924457 date "2018-12-01" @default.
• W2892924457 modified "2023-10-18" @default.
• W2892924457 title "Hydrogen production via natural gas steam reforming in a Pd-Au membrane reactor. Comparison between methane and natural gas steam reforming reactions" @default.
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• W2892924457 doi "https://doi.org/10.1016/j.memsci.2018.09.054" @default.
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