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- W2892961995 endingPage "17690" @default.
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- W2892961995 abstract "Disclosed herein is a visible light mediated cyclization of methyl (α-naphthyl) acrylates and heteroaromatic analogues yielding substituted acenaphthenes and azaacenaphthenes. This highly functional-group-tolerant transformation was put to the test in an enantioselective formal synthesis of delavatine A. Mechanistic details were elucidated by DFT-calculations revealing an unusual intramolecular H-transfer mediated by a primary amine. The generality of this transformation enables a novel synthetic strategy of five membered ring annulation at an advanced stage, allowing reliance upon naphthalene chemistry up to the point of acenaphthene construction." @default.
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- W2892961995 date "2018-10-30" @default.
- W2892961995 modified "2023-09-24" @default.
- W2892961995 title "From Acenaphthenes to (+)-Delavatine A: Visible-Light-Induced Ring Closure of Methyl (α-Naphthyl) Acrylates" @default.
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- W2892961995 doi "https://doi.org/10.1002/chem.201804735" @default.
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