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• W2893088695 abstract "High quality single crystals of ${mathrm{BaBiO}}_{3}$ were grown by congruent melting technique and characterized with x-ray diffraction, x-ray photoemission, and transport property studies. The perovskite oxide ${mathrm{BaBiO}}_{3}$ is a negative charge transfer gap high ${T}_{c}$ oxide parent superconducting compound exhibiting self-doping of holes into the oxygen $2p$ band. We study the low energy scale valence and conduction bands in detail from both a theoretical perspective as well as through x ray, absorption/emission, and photoelectron spectroscopies. X-ray spectroscopy verifies the results of density functional theory (DFT) regarding the overall band structure featuring strong O $2p$ character of the empty antibonding combination of the hybridized Bi $6s$ and O $2p$ states. From the analysis of the core level line shapes we conclude that the dominant O $2p$-Bi $6s$ hybridization energy scale determines the low energy scale electronic structure. This analysis provides further insight into the importance of self-doped oxygen $2p$ states in this high ${T}_{c}$ family of oxides." @default.
• W2893088695 created "2018-10-05" @default.
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• W2893088695 date "2017-10-13" @default.
• W2893088695 modified "2023-10-18" @default.
• W2893088695 title "Experimental and theoretical study of the electronic structure of single-crystal <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mi>BaBiO</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:math>" @default.
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• W2893088695 doi "https://doi.org/10.1103/physrevb.96.165127" @default.
• W2893088695 hasPublicationYear "2017" @default.
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