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- W2893190604 abstract "Abstract Reversible light-modulation of fulgimide based monolayers on Si(1 1 1) and Si(1 0 0) was investigated using ATR-FTIR spectroscopy. Fulgimide monolayers were prepared from neat COOH-terminated SAMs on Si(1 1 1) obtained from methyl undec-10-enoate, (1:1)-diluted COOH-terminated monolayers on Si(1 1 1), and GPTMS monolayers on Si(1 0 0). The epoxy-terminated monolayer on oxidized Si(1 0 0) was characterized with ellipsometry, XPS, as well as contact angle measurements, and ATR-FTIR spectroscopy revealed a strong influence of toluene water content on reproducible high-quality monolayer formation. The results of this study show that environmental polarity has a strong influence on fulgimide imide IR band locations and read-out options for the two photostationary states PSS(365 nm), containing E/Z- and C-isomers, and PSS(545 nm), with solely the E/Z-isomers. Neat COOH-terminated monolayers on flat Si(1 1 1) have the advantage of high functional group concentration, orientation and stability, and an upright arrangement of fulgimide head groups." @default.
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- W2893190604 date "2019-01-01" @default.
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- W2893190604 title "Photoswitching of fulgimides in different environments on silicon surfaces" @default.
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- W2893190604 doi "https://doi.org/10.1016/j.apsusc.2018.09.159" @default.
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