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- W2893229141 abstract "The interfacial behaviour of water remains a central question to fields as diverse as protein folding and surface wetting. Much of our existing knowledge concerning the microscopic motion comes from computational simulation but the dynamics of molecules, on an atomic scale, is largely unexplored by experiment. Here we present experimental results that provide a detailed insight into the behaviour of water monomers on a graphene surface. We show that motion occurs by activated hopping on a primitive lattice that corresponds to the centres of the graphene hexagons. The motion is remarkable because of a strong signature for cooperative behaviour due to repulsive forces between the monomers. The repulsive forces enhance the monomer lifetime ($t_m approx 2$ s at $T_S = 125$ K), providing a precursor gaseous phase that precedes the nucleation of ice islands and, in turn, provides the opportunity for our experiments to be performed. The initial stages of ice growth are generally believed to be dominated by attractive interactions through hydrogen-bonding. Our evidence provides an alternative perspective and suggests that, at least in some cases, nucleation on surfaces may be a process that is kinetically hindered." @default.
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- W2893229141 date "2018-10-01" @default.
- W2893229141 modified "2023-10-18" @default.
- W2893229141 title "Dynamics of water monomers on a hydro-phobic surface" @default.
- W2893229141 hasPublicationYear "2018" @default.
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