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- W2893256185 abstract "Abstract Bulk and surface reconstructed Li[Li0.2Mn0.54Ni0.13Co0.13]O2 cathode materials induced by spinel embedment and γ-MnO2 modification were synthesized by a one-step hydrothermal method. The results of XRD, XPS and SEM confirmed the introduction of γ-MnO2. The analysis of XPS, TEM images, dQ/dV curves and CV curves demonstrated that a spinel phase is embedded synchronously in the bulk of layered structure during the process of γ-MnO2 modification. The results of charge-discharge profiles and dQ/dV curves demonstrated the irreversible discharge capacity loss in the initial cycle is reduced with the introduction and collaboration of spinel and γ-MnO2. Namely, the initial coulombic efficiency is improved up to approximately 100%. Furthermore, the specific discharge capacity and rate performances are enhanced by a structure breakthrough for Li+ transport through blending with electrochemical active spinel-phase and γ-MnO2. In addition, the capacity retention of the material is enhanced from 64% up to 85% after 200 cycles. The main reasons are that the surface of Li[Li0.2Mn0.54Ni0.13Co0.13]O2 is stabilized and the phase transformation from surface to bulk is mitigated under the protection of γ-MnO2 coating layer." @default.
- W2893256185 created "2018-10-05" @default.
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- W2893256185 date "2018-11-01" @default.
- W2893256185 modified "2023-10-02" @default.
- W2893256185 title "Bulk and surface reconstructed Li-rich Mn-based cathode material for lithium ion batteries with eliminating irreversible capacity loss" @default.
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- W2893256185 doi "https://doi.org/10.1016/j.jelechem.2018.09.043" @default.
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