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- W2893498438 abstract "We use coarse-grained (CG) molecular dynamics simulations to determine the effect of uniaxial strain on the stress, scission stress, and scission energy of solutions of wormlike micelles of cetyltrimethylammonium chloride/sodium salicylate (NaSal). We find that the breaking stress, stretch modulus, and scission energy of the charged micelles are nonmonotonic functions of oppositely charged hydrotrope (NaSal) concentration. While the stretch modulus shows a peak at a value of surfactant-to-hydrotrope concentration ratio ( R) close to unity as expected due to neutralization of head-group charge at R = 1, the breaking stress and scission energy produce a peak at R < 1.0 because of thinning of the micelle diameter with increased R. The breaking stress from the simulations depends on the rate of deformation and roughly agrees with the experimental values of Rothstein ( J. Rheol. 2003 , 47 , 1227 ) after extrapolation to the much lower experimental rates. The method and results can be used to predict the effects of flow and mechanical stress on rates of micellar breakage, which is important in the rheology of wormlike micellar solutions." @default.
- W2893498438 created "2018-10-05" @default.
- W2893498438 creator A5029067826 @default.
- W2893498438 creator A5083231687 @default.
- W2893498438 date "2018-09-25" @default.
- W2893498438 modified "2023-09-24" @default.
- W2893498438 title "Stretch and Breakage of Wormlike Micelles under Uniaxial Strain: A Simulation Study and Comparison with Experimental Results" @default.
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- W2893498438 doi "https://doi.org/10.1021/acs.langmuir.8b02421" @default.
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