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- W2893668327 abstract "On the basis of self-consistent field theory (SCFT), we demonstrate that X-shaped rod–coil molecules with hydrogen-bonding groups self-assemble into Archimedean tiling patterns including [36], [44], [63], [3.4.6.4], and [(3.6)2], and dual tiling patterns including dual-[32.4.3.4]. The rod blocks form the edges of polygons, coil blocks fill in the inner spaces of polygons, and the existence of hydrogen bonds further decreases the domain size. A new mechanism is proposed to guide the formation of Archimedean tiling patterns: the fabrication of tiling patterns is controlled by the relationship between the length–diameter ratio β and volume fraction fR of rigid cores in X-shaped supra-macromolecules. This study provides a concept of macromolecular tiling for producing Archimedean tilings and suggests X-shaped rod–coil supra-macromolecules with hydrogen-bonding groups as an ideal platform for the fabrication of two-dimensional nanoscale patterns." @default.
- W2893668327 created "2018-10-05" @default.
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- W2893668327 date "2018-09-26" @default.
- W2893668327 modified "2023-10-18" @default.
- W2893668327 title "Archimedean Tiling Patterns Self-Assembled from X-Shaped Rod–Coil Copolymers with Hydrogen Bonds" @default.
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- W2893668327 doi "https://doi.org/10.1021/acs.macromol.8b01078" @default.
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