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- W2893738169 abstract "Peculiar magnetic behavior was found for 1D-polymeric seven-coordinate pentagonal bipyramidal Fe(II) complex {[Fe(L)(μ1,3-N3)](ClO4)}n (1) with a pentadentate macrocyclic ligand L (3,12,18-triaza-6,9-dioxabicyclo[12.3.1]octadeca-1(18),14,16-triene) coordinated in the pentagonal equatorial plane and with end-to-end bridging azido ligands in axial positions. The static and dynamic magnetic data revealed that spin-canting in the 1D-chain of 1 results in the single-chain magnet (SCM) behavior with high spin-reversal energy barrier Ueff (Δτ) = 87.5 K, exhibiting magnetic hysteresis below 4 K and coexistence with the metamagnetism altogether resulting in weak 3D-ferromagnetic behavior. This is the first reported example of the exclusively azido-bridged homospin Fe(II)-based SCM." @default.
- W2893738169 created "2018-10-05" @default.
- W2893738169 creator A5020987694 @default.
- W2893738169 creator A5063266877 @default.
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- W2893738169 date "2018-09-25" @default.
- W2893738169 modified "2023-10-03" @default.
- W2893738169 title "Single-Chain Magnet Based on 1D Polymeric Azido-Bridged Seven-Coordinate Fe(II) Complex with a Pyridine-Based Macrocyclic Ligand" @default.
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- W2893738169 doi "https://doi.org/10.1021/acs.inorgchem.8b01798" @default.
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- W2893738169 hasPublicationYear "2018" @default.
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