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• W2893825260 abstract "In this work, we found that the open-metal site in a metal–organic framework (MOF) can be used to enhance such selectivity. Hydrogenation of phenylacetylene over such a catalyst enables ultrahigh styrene selectivity of 92% at full conversion with a turnover frequency of 98.1 h–1. The origin of ultrahigh selectivity, as unveiled by density functional theory calculation, is due to a coordination interaction between the open Zn(II) site and the C≡C bond of phenylacetylene." @default.
• W2893825260 created "2018-10-05" @default.
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• W2893825260 date "2018-10-01" @default.
• W2893825260 modified "2023-10-12" @default.
• W2893825260 title "Pd@Zn-MOF-74: Restricting a Guest Molecule by the Open-Metal Site in a Metal–Organic Framework for Selective Semihydrogenation" @default.
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• W2893825260 doi "https://doi.org/10.1021/acs.inorgchem.8b01652" @default.
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