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• W2893827169 abstract "In the present study, photoinduced electron transfer (PET) dynamics between N,N-diethylaniline (DEA) and (E)-9-(4-nitrostyryl)anthracene ( $$hbox {An-NO}_{2}$$ ) in a non-polar solvent medium {methylcyclohexane (MCH)}, has been investigated. The rate constant of back electron transfer ( $$hbox {k}_{{mathrm{BET}}}$$ ) for the $$hbox {An-NO}_{2}$$ – DEA pair was $$sim 3.8times 10^{5}~hbox {s}^{-1}$$ which is ca. 2 orders of magnitude less compared to the anthracene (An)-DEA (control) system. The results indicate that long-lived charge separated species can be generated using the design strategy used herein by achieving resonance stabilization of the excited state (acceptor) radical via conjugation. SYNOPSIS For N,N-diethylaniline/(E)-9-(4-nitrostyryl)anthracene donor-acceptor pair, the back electron transfer rate constant is $$sim 2$$ orders of magnitude slower compared to N,N-diethylaniline/anthracene system. The results indicate that organic molecules with extended $$uppi $$ -conjugation can be utilized for generating long-lived charge separated states via bimolecular PET, due to increased feasibility of charge delocalization." @default.
• W2893827169 created "2018-10-05" @default.
• W2893827169 creator A5022040531 @default.
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• W2893827169 date "2018-09-29" @default.
• W2893827169 modified "2023-09-27" @default.
• W2893827169 title "Photoinduced electron transfer processes of (E)-9-(4-nitrostyryl)anthracene in non-polar solvent medium: generation of long-lived charge-separated states $$^{S }$$ §" @default.
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• W2893827169 doi "https://doi.org/10.1007/s12039-018-1555-8" @default.
• W2893827169 hasPublicationYear "2018" @default.
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