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• W2893885596 abstract "CuO is a promising anode material for lithium-ion batteries due to its high theoretical capacity, low cost, and non-toxicity. However, its practical application has been plagued by low conductivity and poor cyclability. Herein, we report the facile synthesis of porous defective CuO nanosheets by a simple wet-chemical route paired with controlled annealing. The sample obtained after mild heat treatment (300°C) exhibits an improved crystallinity with low dislocation density and preserved porous structure, manifesting superior Li-ion storage capability with high capacity (~500 mAh/g at 0.2 C), excellent rate (175 mAh/g at 2 C), and cyclability (258 mAh/g after 500 cycles at 0.5 C). The enhanced electrochemical performance can be ascribed to the synergy of porous nanosheet morphology and improved crystallinity: (1) porous morphology endows the material a large contact interface for electrolyte impregnation, enriched active sites for Li-ion uptake/release, more room for accommodation of repeated volume variation during lithiation/de-lithiation. (2) the improved crystallinity with reduced edge dislocations can boost the electrical conduction, reducing polarization during charge/discharge. The proposed strategy based on synergic pore and defect engineering can pave the way for development of advanced metal oxides-based electrodes for (beyond) Li-ion batteries." @default.
• W2893885596 created "2018-10-05" @default.
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• W2893885596 date "2018-09-24" @default.
• W2893885596 modified "2023-10-03" @default.
• W2893885596 title "Boosting Lithium-Ion Storage Capability in CuO Nanosheets via Synergistic Engineering of Defects and Pores" @default.
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• W2893885596 doi "https://doi.org/10.3389/fchem.2018.00428" @default.
• W2893885596 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6166579" @default.
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• W2893885596 hasPublicationYear "2018" @default.
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