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- W2893965452 endingPage "6093" @default.
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- W2893965452 abstract "P-Chiral [2.2.1] bicyclic phosphines (HypPhos catalysts) have been applied to reactions between α-alkylallenoates and imines, producing guvacine derivatives. These HypPhos catalysts were assembled from trans-4-hydroxyproline, with the modular nature of the synthesis allowing variations of the exocyclic P and N substituents. Among them, exo-( p-anisyl)-HypPhos was most efficacious for [4 + 2] annulations between ethyl α-methylallenoate and imines. Through this method, ( R)-aplexone was identified as being responsible for the decrease in the cellular levels of cholesterol." @default.
- W2893965452 created "2018-10-05" @default.
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- W2893965452 date "2018-09-24" @default.
- W2893965452 modified "2023-09-29" @default.
- W2893965452 title "Catalytic Enantioselective Synthesis of Guvacine Derivatives through [4 + 2] Annulations of Imines with α-Methylallenoates" @default.
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- W2893965452 doi "https://doi.org/10.1021/acs.orglett.8b02489" @default.
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