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- W2894053511 abstract "Photoreactive composite thin layers with tunable wetting properties from superhydrophilic to superhydrophobic nature were prepared. To achieve extreme wetting properties, the adequate surface roughness is a crucial factor, which was achieved by the incorporation of plasmonic Ag-TiO2 particles, as polymer filler, into the smooth polymer film with adjusted hydrophilicity. The initial copolymer films were synthesized from hydrophilic 2-hydroxyethyl-acrylate (HEA) and hydrophobic perfluorodecyl-acrylate (PFDAc) monomers. In the case of hydrophobic PFDAc, the photocatalyst-roughened thin films displayed superhydrophobic behavior (gamma(tot)(s) similar to 2.3 +/- 1.7 mJ/m(2), Theta > 150 degrees), while the roughened hydrophilic pHEA layers possessed superhydrophilicity (gamma(tot)(s) similar to 72.1 +/- 0.2 mJ/m(2), Theta similar to 0 degrees). The photoactivity of the composites was presented both in solid/gas (S/G) and solid/liquid (S/L) interfaces. According to the light-emitting diode (LED) light photodegradation tests on ethanol (EtOH) as volatile organic compound (VOC) model-molecules at the S/L interface, the superhydrophobic hybrid layer was photooxidized 88.3% of the initial EtOH (0.36 mM). At S/L interface the photocatalytic efficiency was depended on the polarity of the model pollutant molecules: the photooxidation of hydrophobic SUDAN IV (c(0) = 0.25 mg/mL) dye reached 80%, while in the case of the hydrophilic Methylene Blue dye (c(0) = 0.002 mg/mL) it was only 17.3% after 90 min blue LED light (lambda = 405 nm) illumination." @default.
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- W2894053511 date "2018-01-01" @default.
- W2894053511 modified "2023-10-14" @default.
- W2894053511 title "Photoreactive composite coating with composition dependent wetting properties" @default.
- W2894053511 doi "https://doi.org/10.3144/expresspolymlett.2018.93" @default.
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