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• W2894625637 abstract "We demonstrate that a dual frequency comb-transient absorption (DFC-TA) technique can be combined with a time-domain interferometric detection to measure both the transient absorption and refraction spectra of molecules in solution. To do this, the pump–probe signal field of DFC-TA is allowed to interfere with a time-delayed local oscillator field in a time domain. We show that this DFC interferometric pump–probe spectroscopy (DFC-IPS) technique has a unique ability to extract the phase and amplitude information on the pump–probe signal using just a single-scan data, while conventional techniques require an independent signal measured without the pump field for the normalization of the pump–probe spectrum. As a proof-of-principle experiment, we here show that the DFC-IPS enables us to simultaneously measure the frequency-resolved (from 650 to 950 nm) transient absorption and refraction signals with an exceptionally broad dynamic range from femtosecond to nanosecond without using a mechanical translational stage for pump–probe time-scanning. We anticipate that our DFC-IPS technique with femtosecond time-resolution capability will be useful to investigate photoinduced chemical and biological reactions covering broad dynamic ranges." @default.
• W2894625637 created "2018-10-12" @default.
• W2894625637 creator A5027685378 @default.
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• W2894625637 date "2018-10-01" @default.
• W2894625637 modified "2023-10-05" @default.
• W2894625637 title "Interferometric Measurement of Transient Absorption and Refraction Spectra with Dual Frequency Comb" @default.
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• W2894625637 doi "https://doi.org/10.1021/acs.jpcb.8b09262" @default.
• W2894625637 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30273490" @default.
• W2894625637 hasPublicationYear "2018" @default.
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