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• W2894671458 abstract "The adsorption of CO molecules at the Ca3Ru2O7(001) surface was studied using low-temperature scanning tunneling microscopy (STM) and density functional theory (DFT). Ca3Ru2O7 can be easily cleaved along the (001) plane, yielding a smooth, CaO-terminated surface. The STM shows a characteristic pattern with alternating dark and bright stripes, resulting from the tilting of the RuO$_6$ octahedra. At 78,K, CO adsorbs at an apical surface O at the channel edge with a predicted binding energy of $E_{ads} = -0.85$eV. After annealing at room temperature, the CO forms a strong bond ($E_{ads}= -2.04$eV) with the apical O and the resulting carboxylate takes the place of the former surface O. This carboxylate can be decomposed by scanning the surface with a high sample bias voltage of +2.7V, restoring the original surface." @default.
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• W2894671458 date "2019-02-01" @default.
• W2894671458 modified "2023-09-26" @default.
• W2894671458 title "Adsorption of CO on the Ca3Ru2O7(001) surface" @default.
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• W2894671458 doi "https://doi.org/10.1016/j.susc.2018.10.004" @default.
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