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• W2894770903 startingPage "12536" @default.
• W2894770903 abstract "We report the synthesis of a key mononuclear intermediate complex based on a quinoid ligand and its further metalation to afford the corresponding hetero-bimetallic compound that revealed unique properties. An unprecedented hetero-bimetallic effect in coordination chemistry could be indeed observed and exploited to prepare, through selective ligand exchange, a tetranuclear complex (Pd-Ni-Ni-Pd) absorbing light up to the far-red region. Most importantly, we describe here to the best of our knowledge the first use of bischelating ligand for ligand exchange, and this approach can be considered as a new route for incorporating planar units to access multi-heteronuclear complexes. The origin of this specific ligand exchange as well as of the nature of the electronic excited states of the relevant structures were investigated by first-principle calculations." @default.
• W2894770903 created "2018-10-12" @default.
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• W2894770903 date "2018-10-04" @default.
• W2894770903 modified "2023-10-02" @default.
• W2894770903 title "Hetero-Bimetallic Effect as a Route to Access Multinuclear Complexes" @default.
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• W2894770903 doi "https://doi.org/10.1021/acs.inorgchem.8b01466" @default.
• W2894770903 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30285422" @default.
• W2894770903 hasPublicationYear "2018" @default.
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