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- W2894932394 abstract "Strong metal-support interaction (SMSI) has been regarded as one of the most important concepts in heterogeneous catalysis, which has been almost exclusively discussed in metal/oxide catalysts. Here, we show that gold/molybdenum carbide (Au/MoC x) catalysts feature highly dispersed Au overlayers, strong interfacial charge transfer between metal and support, and excellent activity in the low-temperature water-gas shift reaction (LT-WGSR), demonstrating the active SMSI state. Subsequent oxidation treatment results in strong aggregation of Au nanoparticles, weak interfacial electronic interaction, and poor LT-WGSR activity. The two interface states can be transformed into each other by alternative carbonization and oxidation treatments. This work reveals the active SMSI effect in metal/carbide catalysts induced by carbonization, which opens a new territory for this important concept." @default.
- W2894932394 created "2018-10-12" @default.
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- W2894932394 date "2018-10-03" @default.
- W2894932394 modified "2023-10-10" @default.
- W2894932394 title "Carbide-Supported Au Catalysts for Water–Gas Shift Reactions: A New Territory for the Strong Metal–Support Interaction Effect" @default.
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- W2894932394 doi "https://doi.org/10.1021/jacs.8b08246" @default.
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