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• W2894953965 abstract "Layered transition-metal dichalcogenides (TMDs) have provided new opportunities for developing inexpensive and earth-abundant catalysts for electrochemical hydrogen evolution reaction (HER). As the typical family members, semiconducting MoS2 has been widely researched for HER electrocatalysis, while it has been rarely investigated for the emerging metallic VS2, despite high interest and great potential in this area. Herein, by using ultrasmall monolayer MoS2 nanodots as size-controlled precursor, a lamellar heterostructure of MoS2 nanodots and metallic VS2 nanosheets (MoS2 NDs/VS2) is in situ hydrothermally integrated. Via tuning the hybridizing level of MoS2 nanodots, the morphological and structural evolution of the product is explored, and the electrocatalytic HER performances are researched. The optimized hybrid is featured with thinner lamellar heterostructure, upgraded electrical conductivity, increased catalytically active sites and improved intrinsic activity, thus exhibiting significantly enhanced performance for HER electrocatalysis in acidic media. The possible synergistic interaction between the two counterparts is elucidated preliminarily. This work may pave the way for further investigations on TMDs-based heterostructure containing metallic VS2 nanosheets, which shows great potential in broadening the horizon of electrocatalysis and materials chemistry." @default.
• W2894953965 created "2018-10-12" @default.
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• W2894953965 date "2018-10-02" @default.
• W2894953965 modified "2023-10-14" @default.
• W2894953965 title "In Situ Engineering MoS₂ NDs/VS₂ Lamellar Heterostructure for Enhanced Electrocatalytic Hydrogen Evolution" @default.
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• W2894953965 doi "https://doi.org/10.1021/acssuschemeng.8b03929" @default.
• W2894953965 hasPublicationYear "2018" @default.
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