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• W2894964504 abstract "The use of Cerenkov radiation to activate nanoparticles in situ was recently shown to control cancerous tumor growth. Although the methodology has been demonstrated to work, to better understand the mechanistic steps, we developed a mathematic model that integrates Cerenkov physics, light interaction with matter, and photocatalytic reaction engineering. <b>Methods:</b> The model describes a detailed pathway for localized reactive oxygen species (ROS) generation from the Cerenkov radiation–assisted photocatalytic activity of TiO₂. The model predictions were verified by comparison to experimental reports in the literature. The model was then used to investigate the effects of various parameters—the size of TiO₂ nanoparticles, the concentration of TiO₂ nanoparticles, and the activity of the radionuclide ¹⁸F-FDG—on the number of photons and ROS generation. <b>Results:</b> The importance of nanoparticle size in ROS generation for cancerous tumor growth control was elucidated, and an optimal size was proposed. <b>Conclusion:</b> The model described here can be used for other radionuclides and nanoparticles and can provide guidance on the concentration and size of TiO₂ nanoparticles and the radionuclide activity needed for efficient cancer therapy." @default.
• W2894964504 created "2018-10-12" @default.
• W2894964504 creator A5005336166 @default.
• W2894964504 creator A5065659737 @default.
• W2894964504 date "2018-10-05" @default.
• W2894964504 modified "2023-10-16" @default.
• W2894964504 title "Design of Cerenkov Radiation–Assisted Photoactivation of TiO₂ Nanoparticles and Reactive Oxygen Species Generation for Cancer Treatment" @default.
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• W2894964504 doi "https://doi.org/10.2967/jnumed.118.215608" @default.
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