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- W2894971291 abstract "Despite tremendous advances in enantioselective catalysis of the Diels–Alder reaction, the use of simple α,β-unsaturated esters, one of the most abundant and useful class of dienophiles, is still severely limited in scope due to their low reactivity. We report here a catalytic asymmetric Diels–Alder methodology for a large variety of α,β-unsaturated methyl esters and different dienes based on extremely reactive silylium imidodiphosphorimidate (IDPi) Lewis acids. Mechanistic insights from accurate domain-based local pair natural orbital coupled-cluster (DLPNO-CCSD(T)) calculations rationalize the catalyst control and stereochemical outcome." @default.
- W2894971291 created "2018-10-12" @default.
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- W2894971291 date "2018-10-02" @default.
- W2894971291 modified "2023-10-12" @default.
- W2894971291 title "Scalable and Highly Diastereo- and Enantioselective Catalytic Diels–Alder Reaction of α,β-Unsaturated Methyl Esters" @default.
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- W2894971291 doi "https://doi.org/10.1021/jacs.8b07092" @default.
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