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• W2894977987 endingPage "1800640" @default.
• W2894977987 startingPage "1800640" @default.
• W2894977987 abstract "Polymethacrylamide copolymers with hydrophobic N-substituted acrylamides, such as N-cyclohexylacrylamide and N-tert-butylacrylamide, are rare examples of polymers showing composition-dependent thermoresponsive behavior in water. They show unexpected behavior different from the conventional copolymers of a thermoresponsive polymer with hydrophobic comonomers. On increasing the amount of the hydrophobic comonomer in the polymer, there is a change from UCST-type phase behavior to complete solubility, followed by compositions showing LCST-type transition and insolubility in water (U-S-L-I-type change). At 50 mol% of less hydrophobic N-tert-butyl acrylamide (logP 0.87) in contrast to ≈25 mol% of N-cyclohexylacrylamide (logP 1.51), the broad UCST-type transition of polymethacrylamide is turned to LCST-type transitions with very narrow hysteresis in water and PBS buffer. The use of H-bond and water-structure breaker showed the role of H-bonding and hydrophobic interactions in phase transitions of UCST-type and LCST-type, respectively. This work is an important add-on to the infant field of nonionic polymers of UCST-type." @default.
• W2894977987 created "2018-10-12" @default.
• W2894977987 creator A5052481664 @default.
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• W2894977987 date "2018-10-03" @default.
• W2894977987 modified "2023-10-01" @default.
• W2894977987 title "Tuning the Phase Transition from UCST-Type to LCST-Type by Composition Variation of Polymethacrylamide Polymers" @default.
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• W2894977987 doi "https://doi.org/10.1002/marc.201800640" @default.
• W2894977987 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30284344" @default.
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