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- W2895539119 abstract "Precise measurement of the temperature right at the surface of thermoplasmonic nanostructures is a grand challenge but extremely important for the photochemical reaction and photothermal therapy. We present here a method capable of measuring the surface temperature of plasmonic nanostructures with surface-enhanced Raman spectroscopy, which is not achievable by existing methods. We observe a sensitive shift of stretching vibration of a phenyl isocyanide molecule with temperature (0.232 cm–1/°C) as a result of the temperature-dependent molecular orientation change. We develop this phenomenon into a method capable of measuring the surface temperature of Au nanoparticles (NPs) during plasmonic excitation, which is validated by monitoring the laser-induced desorption process of the adsorbed CO on Au NP surface. We further extend the method into a more demanding single living cell thermometry that requires a high spatial resolution, which allows us to successfully monitor the extracellular temperature distribution of a single living cell experiencing cold resistance and the intracellular temperature change during the calcium ion transport process." @default.
- W2895539119 created "2018-10-12" @default.
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- W2895539119 date "2018-10-03" @default.
- W2895539119 modified "2023-10-16" @default.
- W2895539119 title "Quantifying Surface Temperature of Thermoplasmonic Nanostructures" @default.
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- W2895539119 doi "https://doi.org/10.1021/jacs.8b06083" @default.
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- W2895539119 hasPublicationYear "2018" @default.
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