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- W2895643944 abstract "Abstract Hexaphenyl- (1) and hexathienyl-benzene (2) complexes with the six redox-active Cp*(dppe)Fe-C≡C- units are synthesized and their properties in terms of molecular junction are investigated. Both complexes show stepwise multi-redox processes and IVCT bands in the NIR region upon progressive oxidation from the neutral to hexacationic state, as a result of intramolecular electron transfer processes via troidal conjugation through the peripheral aromatic rings. Judging from the Vab values obtained by deconvolution analysis, electronic interaction for thienylene derivative 2 turns out to be stronger than that for the phenylene complex 1. DFT analysis of model complexes support superio'r electron transfer properties for the thienyl derivatives." @default.
- W2895643944 created "2018-10-12" @default.
- W2895643944 creator A5047584152 @default.
- W2895643944 creator A5052492017 @default.
- W2895643944 date "2018-12-01" @default.
- W2895643944 modified "2023-09-24" @default.
- W2895643944 title "Synthesis and intramolecular electronic interactions of hexaarylbenzene bearing redox-active Cp*(dppe)Fe-C≡C- termini" @default.
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- W2895643944 doi "https://doi.org/10.1016/j.jorganchem.2018.10.002" @default.
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