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- W2895812235 abstract "The nucleation mechanisms is of particularly technological interest since it determines the subsequent crystal growth and the resultant performances of glass-ceramics. Here we investigate the temperature dependent nucleation behavior of two compositionally similar silicate glasses. Striking difference in nucleation behavior was found for two glasses containing CaO and MgO, respectively, when they underwent the same heat-treatments under isothermal and non-isothermal conditions. Different from the CaO bearing glass for which only surface nucleation occurs, the substitution of MgO for CaO leads to volume nucleation. The comparison of rheological properties shows that the kinetic term with regard to diffusion makes a weak contribution to this difference in nucleation behavior. In contrast, the topological structure plays a key role in nucleation mechanism, which is strongly affected by the degree of intermediate-range order in both the glasses." @default.
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- W2895812235 date "2019-02-01" @default.
- W2895812235 modified "2023-10-16" @default.
- W2895812235 title "Impact of MgO–CaO substitution on nucleation behaviors of silicate glasses" @default.
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- W2895812235 doi "https://doi.org/10.1016/j.jallcom.2018.10.131" @default.
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