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• W2895861104 startingPage "15022" @default.
• W2895861104 abstract "Herein we report a novel, ozone-based method for postsynthetic generation of mesoporosity in metal-organic frameworks (MOFs). By carefully selecting mixed-ligand Zr-fcu-MOFs based on organic ligand pairs in which one ligand has ozone-cleavable olefin bonds and the other ligand is ozone-resistant, we were able to selectively break the cleavable ligand via ozonolysis to trigger fusion of micropores into mesopores within the MOF framework. This solid-gas phase method is performed at room-temperature, and, depending on the cleavable ligand used, the resultant ligand-fragments can be removed from the ozonated MOF by either washing or sublimation. Compared to the corresponding highly microporous starting MOFs, the highly mesoporous product MOFs exhibit radically distinct gas sorption properties." @default.
• W2895861104 created "2018-10-26" @default.
• W2895861104 creator A5008631097 @default.
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• W2895861104 creator A5081013419 @default.
• W2895861104 date "2018-10-13" @default.
• W2895861104 modified "2023-10-16" @default.
• W2895861104 title "Postsynthetic Selective Ligand Cleavage by Solid–Gas Phase Ozonolysis Fuses Micropores into Mesopores in Metal–Organic Frameworks" @default.
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• W2895861104 doi "https://doi.org/10.1021/jacs.8b09682" @default.
• W2895861104 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30351020" @default.
• W2895861104 hasPublicationYear "2018" @default.
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