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• W2895890437 startingPage "129" @default.
• W2895890437 abstract "Size selected O3−(H2O)n and O2−(H2O)n clusters with n = 0–4, produced by electrospray ionization in a corona discharge, were reacted with CH3Cl in the collision cell of a quadrupole-time-of-flight mass spectrometer under near thermal conditions. The ozonide–water clusters react primarily by ligand exchange, substituting CH3Cl for H2O; dehydration due to collisionally induced dissociation is also observed. Only extremely weak signals are observed for the SN2 reaction between O3−(H2O)n and CH3Cl, yielding Cl−(H2O)n−m, also for the naked ozonide (n = 0). This is in contrast to superoxide–water clusters, where the SN2 reaction with CH3Cl occurs readily. High level quantum chemical computations predict energy barriers in accord with the experimental observations, and the difference in nucleophilicity between O3− and O2− is discussed in light of quantum chemical calculations and Marcus theory." @default.
• W2895890437 created "2018-10-26" @default.
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• W2895890437 date "2019-01-01" @default.
• W2895890437 modified "2023-09-26" @default.
• W2895890437 title "Reactions of microhydrated ozonide with methyl chloride" @default.
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• W2895890437 doi "https://doi.org/10.1016/j.ijms.2018.10.022" @default.
• W2895890437 hasPublicationYear "2019" @default.
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