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- W2895906552 abstract "Hydrogen has emerged as a long-term option for storing energy from renewable resources and has led the scientific community to develop enzyme-inspired catalysts for hydrogen oxidation and production. One of the most productive families of catalysts for H2 oxidation is the pendant amine containing bis(diphosphine)nickel catalysts. Many derivatives of these nickel complexes have been prepared with varying peripheral functionalities to understand their structure–function relationship. Electrocatalysis is currently utilized as the primary tool to measure the catalytic turnover frequencies (TOFs) of these complexes; however, it does not allow accurate determination of TOFs for slow (<1 s–1) to moderately active (∼1–10 s–1) catalysts, and for the slowest catalysts, it can be difficult to determine if they are turning over at all. Further, it does not allow the determination of the TOF in bulk solution. In this work, we demonstrate that a redox chemical procedure involving a change between ferrocenium cation and..." @default.
- W2895906552 created "2018-10-26" @default.
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- W2895906552 date "2018-10-22" @default.
- W2895906552 modified "2023-09-23" @default.
- W2895906552 title "Chemical Method for Evaluating Catalytic Turnover Frequencies (TOF) of Moderate to Slow H<sub>2</sub> Oxidation Electrocatalysts" @default.
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- W2895906552 doi "https://doi.org/10.1021/acs.organomet.8b00580" @default.
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