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- W2895981412 abstract "Conformational isomers are stereoisomers that can interconvert over low potential barriers by rotation around a single bond. However, such bond rotation is hampered by geometrical constraints when molecules are adsorbed on surfaces. Here we show that the adsorption of 4,4'-bis(4-carboxyphenyl)-6,6'-dimethyl-2,2'-bipyridine molecules on surfaces leads to the appearance of pro-chiral single-molecules on NiO(001) and to enantiopure supramolecular domains on Au(111) surfaces containing the $transoid$ molecule conformation. Upon additional Fe adatom deposition, molecules undergo a controlled interconversion from a $transoid$ to $cisoid$ conformation as a result of coordination of the Fe atoms to the 2,2'-bipyridine moieties. As confirmed by atomic force microscopy images and X-ray photoelectron spectroscopy measurements, the resulting molecular structures become irreversibly achiral." @default.
- W2895981412 created "2018-10-26" @default.
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- W2895981412 date "2018-10-09" @default.
- W2895981412 modified "2023-10-06" @default.
- W2895981412 title "Transoid-to-Cisoid Conformation Changes of Single Molecules on Surfaces Triggered by Metal Coordination" @default.
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- W2895981412 doi "https://doi.org/10.1021/acsomega.8b01792" @default.
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