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- W2896429185 abstract "The influence of size-dependent effects on mechanical behavior of a cylindrical silicon electrode particle within a lithium-ion battery is investigated, and it is shown that these effects sensitively determine critical buckling behavior. The mathematical framework used for this investigation incorporates the bond-order-length-strength (BOLS) theory correlation in a general finite deformation theory model that includes the two-way coupling between diffusion-induced stress and stress-influenced diffusion. Additionally, the possibility of plastic flow is accounted for in the model to allow probing situations with relatively high charging rates. Significant differences, arising due to the consideration of the size-dependent effects and captured through the BOLS theory, are highlighted. In particular, it is found that, in most cases studied, both stresses and plastic stretches are amplified in magnitude. Tensile to compressive stress reversal also takes place faster on considering the BOLS theory. The modeling framework is further applied to estimate critical lengths that are safe against buckling. Thus, it is expected that the presented framework will provide an improved aid for the design of nanowire-based lithium ion battery silicon electrodes." @default.
- W2896429185 created "2018-10-26" @default.
- W2896429185 creator A5003182996 @default.
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- W2896429185 date "2018-10-17" @default.
- W2896429185 modified "2023-09-23" @default.
- W2896429185 title "Size-dependent effects sensitively determine buckling of a cylindrical silicon electrode particle in a lithium-ion battery" @default.
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- W2896429185 doi "https://doi.org/10.1063/1.5052236" @default.
- W2896429185 hasPublicationYear "2018" @default.
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