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• W2896750558 endingPage "8267" @default.
• W2896750558 startingPage "8258" @default.
• W2896750558 abstract "We report three types of dicyanodistyrylbenzene (DCS)-based copolymers (PBDT-DCS, PT-DCS, and PNDI-DCS), which present highly balanced ambipolar charge transport characteristics in organic field-effect transistors (OFETs). The introduction of the DCS moiety in a polymer backbone not only lowers the lowest unoccupied molecular orbital (LUMO) level but also increases the crystalline ordering via interchain dipole–dipole interactions. As a result, the LUMO levels for PBDT-DCS, PT-DCS, and PNDI-DCS were decreased to −3.76, −4.00, and −3.99 eV, respectively, which is beneficial for efficient electron injection from Au electrode for improving ambipolar charge transport. The determined hole/electron mobilities of the OFETs were 0.064/0.014, 0.492/0.181, and 0.420/0.447 cm2/(V s) for PBDT-DCS, PT-DCS, and PNDI-DCS, respectively, after thermal annealing at 250 °C. By incorporating the electron-deficient naphthalene diimide (NDI) unit in the copolymers, the n-channel transport was enhanced, with decreasing frontier molecular orbitals with enhanced electron injection and impeded hole injection from the Au electrode. Therefore, PNDI-DCS provided completely symmetric output curves in the positive and negative drain voltage regions with almost equivalent hole and electron mobilities. Benefiting from the balanced ambipolar feature of the PNDI-DCS OFETs, a complementary inverter was successfully fabricated." @default.
• W2896750558 created "2018-10-26" @default.
• W2896750558 creator A5059114171 @default.
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• W2896750558 date "2018-10-10" @default.
• W2896750558 modified "2023-09-28" @default.
• W2896750558 title "Dicyanodistyrylbenzene-Based Copolymers for Ambipolar Organic Field-Effect Transistors with Well-Balanced Hole and Electron Mobilities" @default.
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• W2896750558 doi "https://doi.org/10.1021/acs.macromol.8b01700" @default.
• W2896750558 hasPublicationYear "2018" @default.
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