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- W2896768480 abstract "Functional polyamides are very important polymers that have a variety of valuable applications. However, the effective synthesis of these polymers is still a long-going challenge. Herein, the efficient cyclization of lysine derivative was presented as a universal approach to synthesize e-lactam monomers bearing pendant benzyl-protected hydroxyl, allyloxy, and oligo-ethylene glycol groups. Superbase t-BuP4-catalyzed polymerization could proceed under very mild conditions (e.g., 25 °C) compatible with a wide range of functional pendants, affording high molecular weight (up to 47.7 kg/mol) functional polyamides with high monomer conversion (up to 99%). Of importance, the allyloxy groups were stable toward the initiating and propagating species under mild polymerization conditions. Such an allyloxy-functionalized e-lactam and organocatalytic polymerization to well-defined allylated polyamide has not been reported in the literature and allows further incorporation of an unprecedented range of functional groups..." @default.
- W2896768480 created "2018-10-26" @default.
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- W2896768480 date "2018-10-10" @default.
- W2896768480 modified "2023-10-16" @default.
- W2896768480 title "Functional Polyamides: A Sustainable Access via Lysine Cyclization and Organocatalytic Ring-Opening Polymerization" @default.
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- W2896768480 doi "https://doi.org/10.1021/acs.macromol.8b01790" @default.
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