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- W2896871664 abstract "The earth copious extremely active photo/electrocatalysts have been of immense interest for hydrogen evolution reaction (HER), oxygen evolution reaction (OER) together with environment purification. However, the efficiency of photo/electrocatalysis is still low because of the less visible light absorption and fast recombination of electron-hole pairs. Herein taking the benefits of layered and electronic structural design of Ni-Mn-layered double hydroxide and layered graphitic carbon nitride. A novel Ni-Mn-LDH/g-C3N4 heterostructured photo/electrocatalyst with suited bands was in situ constructed by temperature controlled hydrothermal treatment. A turn in band gap energy within the range of Ni-Mn-LDH to g-C3N4 was noted through a series of physicochemical techniques. Consequently the optimized nanohybrid Ni-Mn-LDH/g-C3N4 (10%) used as best electrocatalyst with JOER = 10 mAcm−2 @ 316 mV and JHER = −60 mAcm−2 @ −147 mV). Furthermore under visible light illumination it function as outperformed photo/electrocatalyst with JOER = 10 mAcm−2 @ 296 mV and JHER = −60 mAcm−2 @ −126 mV in 1 M KOH with a super stability. Similarly it was used for the degradation of RhB with outperformance (≥99%) and rate constant k = 0.313 mn-1. Rivaling the performance of expensive catalysts such as RuO2 and Pt/C and other counterparts. The enhanced photo/electrocatalytic activity ascribed to the formation of band-matched layered by layered heterojunction-accelerated charge separation. It is predicted that our temperature controlled strategy based on earth-profuse elements with structural reliability providing an innovative and inexpensive photo/electrocatalytic system for realistic energy conversion applications." @default.
- W2896871664 created "2018-10-26" @default.
- W2896871664 creator A5002637244 @default.
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- W2896871664 creator A5034170483 @default.
- W2896871664 creator A5043941002 @default.
- W2896871664 creator A5058306675 @default.
- W2896871664 date "2019-03-01" @default.
- W2896871664 modified "2023-10-14" @default.
- W2896871664 title "Layered by layered Ni-Mn-LDH/g-C3N4 nanohybrid for multi-purpose photo/electrocatalysis: Morphology controlled strategy for effective charge carriers separation" @default.
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- W2896871664 doi "https://doi.org/10.1016/j.apcatb.2018.10.005" @default.
- W2896871664 hasPublicationYear "2019" @default.