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• W2897040257 abstract "Several elements of environmental concern are known to exhibit sorption behavior, which is a function of aqueous and mineral surface chemistry. Several surface complexation models (SCM) of differing complexity have been developed based on geochemical principles each of which has its own representation of the mineral/water interface and its own model-specific parameters. These models have been used in a number of environmental studies. To examine the applicability of SCM approaches in performance assessment (PA), it is desirable to generate a set of uniform model-specific SCM parameters that share common reference values. As SCM modeling software and radionuclide thermodynamic data have become more broadly available, current studies have focused on interpreting available radionuclide sorption data to develop the model-specific parameters that describe geochemistry­dependent sorption behavior. In general, an approach that can describe the observed sorption behavior using the simplest models has been adopted. For example, Turner, following approaches developed in Dzombak and Morel, examined the capabilities of the diffuse layer model (DLM), constant capacitance model (CCM), and triple layer model (TLM) to simulate actinide sorption. All three models proved capable of modeling key aspects of observed sorption behavior, although the DLM was able to do so using the fewest parameters. Applied in this manner, a uniform, internally consistent SCM approach can be used to develop a set of parameters based on the common methodologies and reference points, which allows for direct comparison and evaluation of model performance. The surface charge of many minerals varies as a function of pH. SCMs address this pH-dependence assuming an amphoteric surface comprised of hydroxyl groups." @default.
• W2897040257 created "2018-10-26" @default.
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• W2897040257 creator A5021873444 @default.
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• W2897040257 date "2006-01-01" @default.
• W2897040257 modified "2023-09-27" @default.
• W2897040257 title "Applying Surface Complexation Modeling to Radionuclide Sorption" @default.
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• W2897040257 doi "https://doi.org/10.1016/s1573-4285(06)80065-7" @default.
• W2897040257 hasPublicationYear "2006" @default.
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