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• W2897042286 endingPage "15781" @default.
• W2897042286 startingPage "15777" @default.
• W2897042286 abstract "This work demonstrates that the use of high-negative and high-symmetry lacunary polyoxometalates (POMs) for the clustering of alkali metal ions is a feasible strategy not only for the formation of rare high-nuclearity alkali-metal clusters but also for the construction of new-type all-inorganic ionic porous materials. By the strategy, an unprecedented high-nuclearity K-H2 O cluster {K42 (H2 O)60 } with core-shell K6 @K36 configuration is stabilized by 8 C3v -symmetry trivacant POMs [GeW9 O34 ]10- , forming a novel giant ionic alkali-metal-POM composite cluster {K42 Ge8 W72 O272 (H2 O)60 } with more than 100 metal centers. The incorporated 42-nuclearity K-H2 O cluster {K42 (H2 O)60 } exhibits the highest-nuclearity alkali-metal-water cluster known to date in POM chemistry. Further, the giant {K42 Ge8 W72 O272 (H2 O)60 } clusters can be linked by another kind of alkali metal ions Na+ to generate a fascinating three-dimensional all-inorganic ionic porous framework with high chemical stability, proton conductivity, and water vapor adsorption." @default.
• W2897042286 created "2018-10-26" @default.
• W2897042286 creator A5020726667 @default.
• W2897042286 creator A5033865112 @default.
• W2897042286 creator A5046233725 @default.
• W2897042286 creator A5056161767 @default.
• W2897042286 date "2018-10-19" @default.
• W2897042286 modified "2023-10-01" @default.
• W2897042286 title "All-Inorganic Ionic Porous Material Based on Giant Spherical Polyoxometalates Containing Core-Shell K₆ @K₃₆ -Water Cage" @default.
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• W2897042286 doi "https://doi.org/10.1002/anie.201810074" @default.
• W2897042286 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30338895" @default.
• W2897042286 hasPublicationYear "2018" @default.
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